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Smeargle and Sketch is one, but what else?

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Smeargle with Sketch

Chatot with Chatter

Sketch and Chatter the only moves that are truly exclusive to one Pokémon legitimately.

Here is the Link.

Black Kyurem and White Kyurem with Freeze Shock and Ice Burn count here too, because those Moves are yet to be released, but are for those forms.

Pokemon and their Signature Moves

" Volt Tackle - Pichu/Pikachu/Raichu
Pay Day - Meowth/Persian
Kinesis - Kadabra/Alakazam
Barrage - Exeggcute/Exeggutor
Bone Club - Cubone/Marowak
Bonemerang - Cubone/Marowak
Mega Kick - Hitmonlee

Softboiled - Chansey/Blissey*
Lovely Kiss - Jynx
Conversion - Porygon/Porygon2/Porygon-Z
Conversion 2 - Porygon/Porygon2/Porygon-Z
Psystrike - Mewtwo

Octazooka - Octillery
Present - Delibird

Sketch - Smeargle
Triple Kick - Hitmontop
Milk Drink - Miltank
Aeroblast - Lugia
Sacred Fire - Ho-Oh

Smellingsalt - Makuhita/Hariyama
Ice Ball - Spheal/Sealeo/Walrein

Mist Ball - Latias
Luster Purge - Latios
Doom Desire - Jirachi
Psycho Boost - Deoxys

Attack Order - Vespiquen
Defend Order - Vespiquen
Heal Order - Vespiquen
Chatter - Chatot
Roar of Time - Dialga
Spacial Rend - Palkia

Magma Storm - Heatran
Crush Grip - Regigigas
Shadow Force - Giratina*
Lunar Dance - Cresselia
Manaphy - Heart Swap
Darkrai - Dark Void
Seed Flare - Shaymin
Judgement - Arceus

Searing Shot - Victini
V-Create - Victini
Heat Crash - Tepig/Pignite/Emboar
Storm Throw - Throh
Night Daze - Zorua/Zoroark
Tail Slap - Minccino/Cinccino
Horn Leech - Sawsbuck
Electroweb - Joltik/Galvantula

Gear Grind - Klink/Klang/Klinklang
Shift Gear - Klink/Klang/Klinklang
Head Charge - Bouffalant
Fiery Dance - Volcarona
Sacred Sword - Cobalion/Terrakion/Virizion/Keldeo
Fusion Flare - Reshiram
Blue Flare - Reshiram
Fusion Bolt - Zekrom

Bolt Strike - Zekrom
Glaciate - Kyurem
Secret Sword - Keldeo
Relic Song - Meloetta
Techno Blast - Genesect"

Credit to Pokemaster for this information. Good job Pokemaster!

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that is allot of pokemon
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Yes, like Legendaries with their moves. Some non-legends with exclusive moves like,
Exeggcute/Exeggutor w/ Barrage
Jynx w/ Lovely Kiss
For the full list: http://bulbapedia.bulbagarden.net/wiki/Signature_move

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